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Effect of noble metal nanoparticle size on C–N bond cleavage performance in hydrodenitrogenation: a study

Frontiers of Chemical Science and Engineering 2023, Volume 17, Issue 12, Pages 1986-2000 doi: 10.1007/s11705-023-2337-5

Abstract: Breakage of the C–N bond is a structure sensitive process, and the catalyst size significantly affectsobtained by modulating the reduction temperature, and the catalytic activity was evaluated using 1,2,3,4Results showed a 13 times higher reaction rate for sp3sup>-hybridized C–N bond cleavage than sp2sup>-hybridized C–N bond cleavage, while the reaction rate tended to increase first and thenbond cleavage activity, and the step atoms are the active sites for the C–N bond cleavage.

Keywords： sp3sup>/sp2sup>-hybridized C–N bond noble metal nanoparticle catalytic active site turnover

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Calculation of H₂+sup> Structural Parameters based on Hydrogen Atomic Protonized Model

Chen Jing

Strategic Study of CAE 2004, Volume 6, Issue 11, Pages 29-32

Abstract:

The hydrogen atomic protonized model was introduced in present paper for calculation of H₂+sup> structural parameters.Three formulas deduced from above model for bond-length, bond-energy and force constant of hydrogen moleculeion were R_e=2a₀, Keywords： hydrogen molecule ion bond-length bond-energy force constant

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Symbiotic performance, shoot biomass and water-use efficiency of three groundnut (

Sofiya K. MUHABA, Felix D. DAKORA

Frontiers of Agricultural Science and Engineering 2020, Volume 7, Issue 4, Pages 455-466 doi: 10.15302/J-FASE-2020354

Abstract: fixation, and C assimilation.There was, however, no effect on shoot δ C values in either year.The three genotypes differed significantly in δ N, %Ndfa, N-fixed, grain yield, C concentration, and δ C.soil N uptake.

Keywords： shoot yield N-fixed %Ndfa δ15sup>N δ13sup>C water-use efficiency

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Removal of ammonium and nitrate through Anammox and FeS-driven autotrophic denitrification

Frontiers of Environmental Science & Engineering 2023, Volume 17, Issue 6, doi: 10.1007/s11783-023-1674-4

Abstract:

● Simultaneous NH₄+sup>/NO₃–sup

Keywords： Anammox Denitrification FeS NH₄+sup>/NO₃−sup> Sulfammox

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An electrochemical process that uses an Fe

Chaojie Jiang, Lifen Liu, John C. Crittenden

Frontiers of Environmental Science & Engineering 2016, Volume 10, Issue 4, doi: 10.1007/s11783-016-0860-z

Abstract: A bio-electrochemical fuel cell reactor with cathodic Fe /TiO generates electricity. It destroys recalcitrant pollutants in cathode chamber without photocatalysis. Fe /TiO generates reactive oxygenated species in the dark or under photocatalysis. Cathodic produced ROS (hydroxy radical/superoxide radical) can degrade tetracycline or dyes. Electricity generation is enhanced by semiconductor catalyzed cathodic degradation of pollutants. In this study, a new water treatment system that couples (photo-) electrochemical catalysis (PEC or EC) in a microbial fuel cell (MFC) was configured using a stainless-steel (SS) cathode coated with Fe /TiO . We examined the destruction of methylene blue (MB) and tetracycline. Fe /TiO was prepared using a chemical reduction-deposition method and coated onto an SS wire mesh (500 mesh) using a sol technique. The anode generates electricity using microbes (bio-anode). Connected via wire and ohmic resistance, the system requires a short reaction time and operates at a low cost by effectively removing 94% MB (initial concentration 20 mg·L ) and 83% TOC/TOC under visible light illumination (50 W; 1.99 mW·cm for 120 min, MFC-PEC). The removal was similar even without light irradiation (MFC-EC). The of the MFC-PEC system was approximately 0.675 kWh·m ·order , whereas that of the MFC-EC system was zero. The system was able to remove 70% COD in tetracycline solution (initial tetracycline concentration 100 mg·L ) after 120 min of visible light illumination; without light, the removal was 15% lower. The destruction of MB and tetracycline in both traditional photocatalysis and photoelectrocatalysis systems was notably low. The electron spin-resonance spectroscopy (ESR) study demonstrated that ·OH was formed under visible light, and ·O was formed without light. The bio-electricity-activated O and ROS (reactive oxidizing species) generation by Fe /TiO effectively degraded the pollutants. This cathodic degradation improved the electricity generation by accepting and consuming more electrons from the bio-anode.

Keywords： Bio-anode Photocatalytic cathode Fe0sup>/TiO₂ ESR Dye and antibiotics Advanced oxidation

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Selective recovery of Cu

Haiping LUO,Bangyu QIN,Guangli LIU,Renduo ZHANG,Yabo TANG,Yanping HOU

Frontiers of Environmental Science & Engineering 2015, Volume 9, Issue 3, Pages 522-527 doi: 10.1007/s11783-014-0633-5

Abstract: As the bioelectrochemical system, the microbial fuel cell (MFC) and the microbial electrolysis cell (MEC) were developed to selectively recover Cu and Ni ions from wastewater. The wastewater was treated in the cathode chambers of the system, in which Cu and Ni ions were removed by using the MFC and the MEC, respectively. At an initial Cu concentration of 500 mg·L , removal efficiencies of Cu increased from 97.0%±1.8% to 99.0%±0.3% with the initial Ni concentrations from 250 to 1000 mg·L , and maximum power densities increased from 3.1±0.5 to 5.4±0.6 W·m . The Ni removal mass in the MEC increased from 6.8±0.2 to 20.5±1.5 mg with the increase of Ni concentrations. At an initial Ni concentration of 500 mg·L , Cu removal efficiencies decreased from 99.1%±0.3% to 74.2%±3.8% with the initial Cu concentrations from 250 to 1000 mg·L , and maximum power densities increased from 3.0±0.1 to 6.3±1.2 W·m . Subsequently, the Ni removal efficiencies decreased from 96.9%±3.1% to 73.3%±5.4%. The results clearly demonstrated the feasibility of selective recovery of Cu and Ni from the wastewater using the bioelectrochemical system.

Keywords： bioelectrochemical system Cu2+sup> Ni2+sup> selective recovery

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Metal-Free Hexagonal Perovskite High-Energetic Materials with NH₃OH+sup>/NH₂NH₃+sup> as B-site Cations Article

Yu Shang, Zhi-Hong Yu, Rui-Kang Huang, Shao-Li Chen, De-Xuan Liu, Xiao-Xian Chen, Wei-Xiong Zhang, Xiao-Ming Chen

Engineering 2020, Volume 6, Issue 9, Pages 1013-1018 doi: 10.1016/j.eng.2020.05.018

Abstract: /sub>dabco)B(ClO₄)₃ (H₂dabco2+sup> = 1,4-diazabicyclo[2.2.2]octane-1,4-diium), were fabricated via an easily scaled-up synthetic route using NH₃OH+sup> and NH₂NH₃+sup> as B-site cations, respectively.Compared with their NH₄+sup> analog ((H₂dabco)(NH₄)(ClO_{4has an ultrahigh thermal stability (decomposition temperatures (T_d) = 375.3 °C)}

Keywords： Energetic materials Single explosive Solid propellant Metal-free Hexagonal perovskite

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Innate and adaptive T cells in influenza disease

Simone Nüssing, Sneha Sant, Marios Koutsakos, Kanta Subbarao, Thi H.O. Nguyen, Katherine Kedzierska

Frontiers of Medicine 2018, Volume 12, Issue 1, Pages 34-47 doi: 10.1007/s11684-017-0606-8

Abstract: summarize the current knowledge on influenza-specific innate MAIT and gd T cells as well as adaptive CD8+sup> and CD4+sup> T cells, and discuss how these responses can be harnessed by novel vaccine

Keywords： influenza innate T cells CD4+sup> and CD8+sup> T cells vaccination

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NETO2 promotes melanoma progression via activation of the Ca/CaMKII signaling pathway

Frontiers of Medicine 2023, Volume 17, Issue 2, Pages 263-274 doi: 10.1007/s11684-022-0935-0

Abstract: Neuropilin and tolloid-like 2 (NETO2) is closely related to tumorigenesis.However, the functional significance of NETO2 in melanoma progression remains unclear.invasion by downregulating the levels of calcium ions (Ca2+sup>) and the expression of key genesBy contrast, NETO2 overexpression had the opposite effects.indicating that targeting NETO2 may effectively improve melanoma treatment.

Keywords： melanoma neuropilin and tolloid-like 2 Ca2+sup>/CaMKII signaling pathway

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Effects of La, Ce on nitrogen removal in sequencing batch reactor

Qing XIA , Rui LIANG , Yuning HONG , Lili DING , Hongqiang REN , Yuxiang MAO , Mingyu ZHAO ,

Frontiers of Environmental Science & Engineering 2009, Volume 3, Issue 3, Pages 369-374 doi: 10.1007/s11783-009-0036-1

Abstract: The data showed that higher NH―N removal rate, total inorganic nitrogen removal efficiency, andof SBR, the presence of REEs increased the total inorganic nitrogen removal efficiency and NH―N

Keywords： rare earth La3+sup> Ce3+sup> inorganic nitrogen nitrogen removal sequencing batch reactor

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Study on Algorithm A*sup> Based on Dynamic Representation of Binary Tree for Environment and Robotic

Tang Ping,Yang Yimin

Strategic Study of CAE 2002, Volume 4, Issue 9, Pages 50-53

Abstract: A new algorithm A*sup> , which plans the path of soccer robots in complicated environments is

Keywords： dynamic binary-tree algorithm A*sup> path planning

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Clinical significance of CD34+sup>CD117dimsup>/CD34+sup>CD117brisup> myeloblast-associated

Xueping Li, Yuting Dai, Bing Chen, Jinyan Huang, Saijuan Chen, Lu Jiang

Frontiers of Medicine 2021, Volume 15, Issue 4, Pages 608-620 doi: 10.1007/s11684-021-0836-7

Abstract: t(8;21)(q22;q22) acute myeloid leukemia (AML) is a highly heterogeneous hematological malignancy with a high relapse rate in China. Two leukemic myeloblast populations (CD34 CD117 and CD34 CD117 ) were previously identified in t(8;21) AML, and CD34 CD117 cell proportion was determined as an independent factor for this disease outcome. Here, we examined the impact of CD34 CD117 /CD34 CD117 myeloblast-associated gene expression on t(8;21) AML clinical prognosis. In this study, 85 patients with t(8;21) AML were enrolled. The mRNA expression levels of CD34 CD117 -associated genes ( , , and ) and CD34 CD117 -associated genes ( , , and ) were measured using quantitative reverse transcription PCR. Associations between gene expression and clinical outcomes were determined using Cox regression models. Results showed that patients with high , , or expression had significantly inferior overall survival (OS), whereas those with high or expression showed relatively favorable prognosis. Univariate analysis revealed that CD19, CD34 CD117 proportion, mutation, minimal residual disease (MRD), and expression levels of , , , and were associated with OS. Multivariate analysis indicated that mutation, MRD and and expression levels were independent prognostic variables for OS. Identifying the clinical relevance of CD34 CD117 /CD34 CD117 myeloblast-associated gene expression may provide new clinically prognostic markers for t(8;21) AML.

Keywords： t(8 21)(q22 q22) AML CD34+sup>CD117dimsup>/ CD34+sup>CD117brisup> cell population

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K+sup> and Na+sup> fluxes in roots of two Chinese Iris populations

Pinfang LI,Biao ZHANG

Frontiers of Agricultural Science and Engineering 2014, Volume 1, Issue 2, Pages 144-149 doi: 10.15302/J-FASE-2014016

Abstract: Maintenance of ion homeostasis, particularly the regulation of K and Na uptake, is important for all plants to adapt to salinity. Observations on ionic response to salinity and net fluxes of K , Na in the root exhibited by plants during salt stress have highlighted the need for further investigation. The objectives of this study were to compare salt adaptation of two Chinese Iris ( Pall. var. (Fisch.) Koidz.) populations, and to improve understanding of adaptation to salinity exhibited by plants. Plants used in this study were grown from seeds collected in the Xinjiang Uygur Autonomous Region (Xj) and Beijing Municipality (Bj), China. Hydroponically-grown seedlings of the two populations were supplied with nutrient solutions containing 0.1 (control) and 140 mmol·L NaCl. After 12 days, plants were harvested for determination of relative growth rate and K , Na concentrations. Net fluxes of K , Na from the apex and along the root axis to 10.8 mm were measured using non-invasive micro-test technique. With 140 mmol·L NaCl treatment, shoots for population Xj had larger relative growth rate and higher K concentration than shoots for population Bj. However, the Na concentrations in both shoots and roots were lower for Xj than those for Bj. There was a lower net efflux of K found in population Xj than by Bj in the mature zone (approximately 2.4-10.8 mm from root tip). However, no difference in the efflux of Na between the populations was obtained. Population Xj of continued to grow normally under NaCl stress, and maintained a higher K /Na ratio in the shoots. These traits, which were associated with lower K leakage, help population Xj adapt to saline environments.

Keywords： Koidz population K+sup> and Na+sup> ion flux non-invasive micro-test technique

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Genetic variants in the ADD1 and GNB3 genes and blood pressure response to potassium supplementation

JAQUISH PhD, Dabeeru C. RAO PhD, Charles GU PhD, James E.HIXSON PhD, Chung-Shiuan CHEN MS8sup>, Paul K. WHELTON MD, MSc9sup>,

Frontiers of Medicine 2010, Volume 4, Issue 1, Pages 59-66 doi: 10.1007/s11684-010-0015-8

Abstract: ) in the adducin 1 alpha (ADD1) and guanine nucleotide binding protein (G protein) beta polypeptide 3(GNB3) genes and systolic BP (SBP), diastolic BP (DBP), and mean arterial pressure (MAP) responses to

Keywords： potassium potassium sensitivity adducin 1 alpha (ADD1) guanine nucleotide binding protein beta polypeptide 3(GNB3)

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Facile synthesis and enhanced visible-light photocatalytic activity of Ti

Xiaojie Zhang,Lei Wang,Shuqing Chen,Yi Huang,Zhuonan Song,Miao Yu

Frontiers of Chemical Science and Engineering 2015, Volume 9, Issue 3, Pages 349-358 doi: 10.1007/s11705-015-1523-5

Abstract: Ti -doped TiO nanosheets with tunable phase composition (doped TiO (A/R)) were synthesized via a hydrothermal method with high surface area anatase TiO nanosheets TiO (A) as a substrate, structure directing agent, and inhibitor; the activity was evaluated using a probe reaction-photocatalytic CO conversion to methane under visible light irradiation with H as an electron donor and hydrogen source. High-resolution transmission electron microscope (HRTEM), field emission scanning electron microscope, UV-Vis diffuse reflectance spectra, and X-ray diffraction (XRD) etc., were used to characterize the photocatalysts. XRD and HRTEM measurements confirmed the existence of anatase-rutile phase junction, while Ti and single-electron-trapped oxygen vacancy in the doped TiO (A/R) photocatalyst were revealed byelectron paramagnetic resonance (EPR) measurements. Effects of hydrothermal synthesis temperature and the amount of added anatase TiO on the photocatalytic activity were elucidated. Significantly enhanced photocatalytic activity of doped TiO (A/R) was observed; under the optimized synthesis conditions, CH generation rate of doped TiO (A/R) was 2.3 times that of Ti -doped rutile TiO .

Keywords： Ti3+sup>-doped TiO₂ photocatalytic CO₂ conversion visible light irradiation

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Title Author Date Type Operation

Effect of noble metal nanoparticle size on C–N bond cleavage performance in hydrodenitrogenation: a study

Journal Article

Calculation of H₂+sup> Structural Parameters based on Hydrogen Atomic Protonized Model

Chen Jing

Journal Article

Symbiotic performance, shoot biomass and water-use efficiency of three groundnut (

Sofiya K. MUHABA, Felix D. DAKORA

Journal Article

Removal of ammonium and nitrate through Anammox and FeS-driven autotrophic denitrification

Journal Article

An electrochemical process that uses an Fe

Chaojie Jiang, Lifen Liu, John C. Crittenden

Journal Article

Selective recovery of Cu

Haiping LUO,Bangyu QIN,Guangli LIU,Renduo ZHANG,Yabo TANG,Yanping HOU

Journal Article

Metal-Free Hexagonal Perovskite High-Energetic Materials with NH₃OH+sup>/NH₂NH₃+sup> as B-site Cations

Yu Shang, Zhi-Hong Yu, Rui-Kang Huang, Shao-Li Chen, De-Xuan Liu, Xiao-Xian Chen, Wei-Xiong Zhang, Xiao-Ming Chen

Journal Article

Innate and adaptive T cells in influenza disease

Simone Nüssing, Sneha Sant, Marios Koutsakos, Kanta Subbarao, Thi H.O. Nguyen, Katherine Kedzierska

Journal Article

NETO2 promotes melanoma progression via activation of the Ca/CaMKII signaling pathway

Journal Article

Effects of La, Ce on nitrogen removal in sequencing batch reactor

Qing XIA , Rui LIANG , Yuning HONG , Lili DING , Hongqiang REN , Yuxiang MAO , Mingyu ZHAO ,

Journal Article

Study on Algorithm A*sup> Based on Dynamic Representation of Binary Tree for Environment and Robotic

Tang Ping,Yang Yimin

Journal Article

Clinical significance of CD34+sup>CD117dimsup>/CD34+sup>CD117brisup> myeloblast-associated

Xueping Li, Yuting Dai, Bing Chen, Jinyan Huang, Saijuan Chen, Lu Jiang

Journal Article

K+sup> and Na+sup> fluxes in roots of two Chinese Iris populations

Pinfang LI,Biao ZHANG

Journal Article

Genetic variants in the ADD1 and GNB3 genes and blood pressure response to potassium supplementation

JAQUISH PhD, Dabeeru C. RAO PhD, Charles GU PhD, James E.HIXSON PhD, Chung-Shiuan CHEN MS8sup>, Paul K. WHELTON MD, MSc9sup>,

Journal Article

Facile synthesis and enhanced visible-light photocatalytic activity of Ti

Xiaojie Zhang,Lei Wang,Shuqing Chen,Yi Huang,Zhuonan Song,Miao Yu

Journal Article

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